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Dataset / Data from: Temperature Dependence of Sea Spray Aerosol Production

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Title
Data from: Temperature Dependence of Sea Spray Aerosol Production
Creator
Cappa, Chris D
Date Created and/or Issued
2015-07-01 to 2018-04-01
Contributing Institution
UC San Diego, Research Data Curation Program
Collection
Center for Aerosol Impacts on Chemistry of the Environment (CAICE)
Rights Information
Under copyright
Constraint(s) on Use: This work is protected by the U.S. Copyright Law (Title 17, U.S.C.). Use of this work beyond that allowed by "fair use" or any license applied to this work requires written permission of the copyright holder(s). Responsibility for obtaining permissions and any use and distribution of this work rests exclusively with the user and not the UC San Diego Library. Inquiries can be made to the UC San Diego Library program having custody of the work.
Use: This work is available from the UC San Diego Library. This digital copy of the work is intended to support research, teaching, and private study.
Rights Holder and Contact
UC Regents
Description
Publication abstract: The dependence of sea spray aerosol (SSA) particle number concentrations (Np) and size distributions on water temperature (Tw) over the range 2-25°C was quantified for particles generated from both a marine aerosol reference tank (MART) and a miniature MART (miniMART). Four water types were considered: NaCl water, reef salt (RS) water, filtered and autoclaved reef salt (FARS), and filtered but not autoclaved seawater (NASW). For NaCl, RS, and FARS water the Np exhibited a moderate, monotonic increase with Tw, with a sensitivity of 1.0 – 3.3% °C-1. This contrasts with some previous laboratory studies that used alternative generation methods but is consistent with determinations and parameterizations that are based on ambient observations. Complementary experiments using a continuous plunging jet with FARS water yield the same Tw dependence as MART and miniMART experiments suggesting that differences in particle generation method cannot explain the different results here compared to literature studies. The number-weighted size distributions here consisted of two modes. The larger mode exhibited a stronger Tw-dependence, although the overall shape was relatively insensitive to Tw. The Tw-sensitivity of Np for actual seawater (NASW) differed from the other water types, exhibiting complex, irreproducible behavior due most likely to temporally evolving seawater composition. These observations provide new constraints and context for understanding the dependence of SSA production on water temperature and composition.
Research Data Curation Program, UC San Diego, La Jolla, 92093-0175 (https://lib.ucsd.edu/rdcp)
Forestieri, Sara D.; Moore, Kathryn A.; Martinez, Rosemarie; Wang, Alex; Stokes, M. D.; Cappa, Chris D. (2018). Data From: Temperature Dependence of Sea Spray Aerosol Production. In Center for Aerosol Impacts on Chemistry of the Environment (CAICE). UC San Diego Library Digital Collections. https://doi.org/10.6075/J03J3B5D
Type
dataset
Identifier
ark:/20775/bb01059646
Subject
Ocean emissions
Sea spray aerosol (SSA)
Aerosol particles

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